I believe you want to use the ADDMEDIBRM command. Here is the HELP text from this command:
The Add Media Information to BRM (ADDMEDIBRM) command adds file level detail to the BRMS media inventory content volume information. The files and the volumes that contain them can be from another tape inventory or from some other outside source. The purpose of the command is to allow user applications or another volume management system to insert data (volume file descriptions) into the BRMS media contents information so that the volumes and their contents can be managed. The volume for which you are adding content information must exist in the media inventory and the volume, file sequence and volume sequence must be unique in the BRMS media inventory contents information. Multiple volumes will write a media information record for each volume with the volume sequence being increased as the records are added.
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This was first published in May 2004